Enhancement of Rb Fine-Structure Transfer in 4He Due to Three-Body Collisions

Document Type

Article

Publication Date

7-1-2010

Department

Physics and Astronomy

School

Mathematics and Natural Sciences

Abstract

Using ultrafast laser excitation and time-correlated single-photon counting techniques, we have measured the collisional mixing rates between the rubidium 52P fine-structure levels in the presence of 4He gas. A nonlinear dependence of the mixing rate with 4He density is observed. We find Rb fine-structure transfer is primarily due to binary collisions at 4He densities of ≤1019cm-3, while at greater densities, three-body collisions become significant. We determine a three-body collisional transfer rate coefficient (52P3/2 → 52P1/2) of 1.25(9) × 10-32cm6/s at 22°C.

Publication Title

Optics Letters

Volume

35

Issue

13

First Page

2146

Last Page

2148

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